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relationship for the flow velocity as a function of the spatial coordinates (i.e. solution of Eq. (2.7.8) with suitable boundary conditions) and (b) Solution of Eq. (2.7.6) or Eq. (2.7.7) on the basis of a known relationship for v, or for vx, vy and vz This approach is possible only if density gradients are not formed in the solution as a result of transport processes (e.g. in dilute solutions). Otherwise, both differential equations must be solved simultaneously a very difficult task. Two examples will now be given of solution of the convective diffusion problem, transport to a rotating disk as a stationary case and transport to a growing sphere as a transient case. Finally, an engineering approach will be mentioned in which the solution is expressed as a function of dimensionless quantities characterizing the properties of the system. As a rotating disk is a very useful device for many types of electrochemical research, convective diffusion to a rotating disk, treated theoretically by V. G. Levich, will be used here as an example of this type of transport process. Consider a disk in the xz plane, rotating around the y axis with radial velocity co (see Fig. 2.22). If the radius of the disk is sufficiently larger

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probe light. With UV light (B20 mW/cm2) turned on for 5 s, the trans cis isomerization of azobenzene is enough to induce the nematic isotropic phase transition, resulting in the drop of diffraction ef ciency. Subsequently, after 5 s of visible light exposure (B26 mW/cm2), the high diffraction state is recovered,

Fig. 2.22 Distribution of streamlines of the liquid at the surface of a rotating disk. Above: a side view; below: a view from the direction of the disk axis. (According to V. G. Levich)

because the cis trans backisomerization of azobenzene allows the oriented nematic phase to be recovered Under the used 5-s irradiation, the actual diffraction drop and recovery times are B34 and 14 s, respectively Similar to electrical switching, the optical switching can be realized for many cycles without signi cant degradation of switching performance From the switching mechanism, it is easy to understand that under UV light, the switching speed is determined by the rate of the photochemical nematic isotropic phase transition The reverse switching under the action of visible light is determined by the isotropic nematic phase transition and the concurrent reorientation of LC molecules induced by rubbed surfaces Increasing the intensities of UV and visible lights can increase the speed of optical switching.

139 than the thickness of the hydrodynamic layer, then the change of flow at the edge of the disk can be neglected. Solution of the hydrodynamic part of the problem, carried out by von Karman and Cochrane, indicates that the thickness of the hydrodynamic layer is not a function of the distance from the centre of the disk y; its value in centimetres is given by the relationship

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(2.7.9) The velocity of the liquid in the direction perpendicular to the surface of the disk in centimetres per second is described by the equation vy = -0.51co3/2y-y2y2 (2.7.10)

The similar low and high diffraction ef ciencies for both electrical and optical switching are in accordance with the analysis of the index modulation changes as discussed in Fig 1124 The results thus con rm that both an electrical eld and light at two wavelengths can be used to switch reversibly the diffraction ef ciency of gratings prepared using the designed azobenzene polymer-stabilized LCs For both modes of switching, varying the voltage or the intensity of light can switch the diffraction ef ciency to different levels While a voltage needs to be held constantly to keep the low diffraction state, the use of UV light requires no continuous excitation But in the latter case, the stability is limited by the thermally induced cis trans backisomerization For the LC azobenzene monomer used, the thermal relaxation of the cis isomer is slow, taking hours to complete in solution.

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It will be assumed that the concentration gradient in the direction perpendicular to the surface of the disk is much greater than in the radial direction. Then Eq. (2.7.7) reduces to the form dc _ The boundary conditions are