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Each sort of complex including the free ions has a characteristic electrode reaction rate constant (for example, kcMX., / = 0, 1,. . ., n). Consider the relatively simple case where the chemical reactions of formation and dissociation of the complexes are sufficiently fast so that equilibrium among the complexes, free ions and complexing agent is maintained everywhere in the electrolyte during the electrolysis. The rate of deposition of the metal is then determined by the electrode reaction of the complex MX,-, for which the product kcMX.cMX. is, at the given potential, the largest for all the complexes. 5.6.3 Chemical volume reactions According to the theory developed by R. Brdicka and K. Wiesner, a chemical reaction prior to the electrode reaction acts as the rate-controlling step in the electrode process when the electrode reaction disturbs the chemical equilibrium in solution and renewal of this equilibrium is not sufficiently fast. This effect extends to a certain depth in the solution as concentration changes resulting from the electrode reaction are propagated by diffusion. According to J. Koutecky and R. Brdicka, the differential equation describing diffusion to an electrode with a simultaneous chemical reaction is given by combination of the second Fick law and the equation for the reaction rate (this idea first appeared in a paper by A. Eucken). Consider a system of two substances participating in a reversible reaction B <= A (5.6.9)

Scheme 12.7 Preparation of azo BCs by supramolecular self-assembly between a BC and a low molecular weight azo compound. Source: Reproduced from Sidorenko et al., 2003.

After a data center has been implemented using the hot aisle/cold aisle concept, one of the most common problems is bypass airflow. This means that the cool air is not getting to the air intakes of the computer equipment, but is instead bypassing the intended route through leaks, cable cutouts, holes under cabinets, or improperly placed vented tiles. Bypass airflow can be avoided easily, through the following tips as recommended by experts such as the Uptime Institute, APC, and Liebert:

with the equilibrium constant K = k2/kl. The substance A is present in a marked excess over substance B (K 1), so that its concentration is practically not changed by the electrode process. The substance B undergoes an irreversible electrode reaction with the rate constant kc = k^ exp [ - anF(E - E ')/RT] (see Eq. 5.2.23). The differential equation and boundary and initial conditions for substance B are dc d^c = D f + Jt^CA-ZCce)

Some special reaction with a particularly designed route can be used to synthesize azo BCs. For instance, a series of poly(vinyl ether)-based azo LCBCs were synthesized by using living cationic polymerization and free-radical polymerization techniques (Serhatli and Serhatli, 1998). As shown in Scheme 12.8, 4.4uazobis(4-cyano pentanol) (ACP) was used to couple quantitatively two wellde ned polymers of LC living poly(vinyl ether), initiated by the methyl tri uoromethane sulfonate/tetrahydrothiophene system. Then the ACP in the main chain was thermally decomposed to produce polymeric radical, which was used to initiate the polymerization of MMA or styrene to obtain PMMA-based or PS-based azo BCs (AB or ABA types).

Ta(110) Ta(lll) Ta(lll)

Seal all the holes in the computer-room perimeter. Seal all openings in the raised floor to prevent bypass cold-air flow (cable cutouts, PDUs [power-distribution units] and cooling units, floor edges, cutouts for pipes, and so on). Install blanking plates in all unused spaces in equipment racks and cabinets to prevent recirculation of hot air. Continued

Azo BCs are multifunctional polymeric materials, which combine the photochemical properties of azo polymers and the microphase separation of functional BCs. On the one hand, the azo block and the other segments cannot be miscible, unlike statistically random copolymers in which the azo moieties are dispersed homogeneously over the whole bulk lms. On the other hand, the azo BCs cannot form macroscopically phase-separated structures like polymer blends (Bates and Fredrichson, 1999). The azo moiety may play the roles of both mesogen and photosensitive chromophore, when it is attached to the polymer main chain by a longer soft spacer. Both the photoisomerization and the phase transition of the LC to the isotropic phase are involved in the process of microphase separation because of